I'm afraid not. They are barely in it. Crowley dies in the beginning of Season 3 tragically, because of pies, and Aziraphale also dies in Season 3 but hilariously, because of falling in a hole.

The rest of Season 3 is a story about three little rabbits who go to the big city to open a conveyor belt sushi restaurant, and their family's involvement with the East German secret police in the early 1960s.